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As part of the process to add @charlotte.edu addresses to University email accounts, your default send as address will be changed to an @charlotte.edu address.
In the window that opens, type your email@example.com address in the Email address: field then click Next Step
Your name should already show in the Name field. The Treat as an alias checkbox should remain checked.
You will now see your firstname.lastname@example.org address listed in the Send mail as: section
If you already have email@example.com as your default send as address, you will not be able to permanently set your firstname.lastname@example.org address to the default. The default send as address is administratively synced which will overwrite any change you try to make to your default send as address.